Heat transport of the kagome Heisenberg quantum spin liquid candidate <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>YCu</mml:mi><mml:mn>3</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:mi>OH</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mrow><mml:mn>6.5</mml:mn></mml:mrow></mml:msub><mml:msub><mml:mi>Br</mml:mi><mml:mrow><mml:mn>2.5</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math> : Localized magnetic excitations and a putative spin gap

نویسندگان

چکیده

The spin-1/2 kagom\'{e} Heisenberg antiferromagnet is generally accepted as one of the most promising two-dimensional models to realize a quantum spin liquid state. Previous experimental efforts were almost exclusively on only archetypal material, herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, which unfortunately suffers from notorious orphan spins problem caused by magnetic disorders. Here we turn YCu$_3$(OH)$_{6.5}$Br$_{2.5}$, recently recognized another host globally undistorted Cu$^{2+}$ lattice free spins, thus more feasible system for studying intrinsic physics. Our high-resolution low-temperature thermal conductivity measurements yield vanishing small residual linear term $\kappa/T$ ($T\rightarrow 0$), and clearly rule out itinerant gapless fermionic excitations. Unusual scattering phonons grows exponentially with temperature, suggesting thermally activated phonon-spin hence gapped excitation, consistent $\mathbb{Z}_2$ ground Additionally, analysis field impact reveals closing gap, while excitations remain localized.

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ژورنال

عنوان ژورنال: Physical Review B

سال: 2022

ISSN: ['1098-0121', '1550-235X', '1538-4489']

DOI: https://doi.org/10.1103/physrevb.106.l220406